Angelina Jolie Films as Brad Pitt Lobbies in Washington D.C.

Angelina Jolie and Brad Pitt are taking over the nation's capital.

Clad in a black beanie and camel-colored coat, Jolie, 33, filmed her upcoming CIA thriller Salt in Washington D.C. on Thursday morning. According to The Washington Post, production was delayed by bad weather Wednesday at the Mandarin Oriental hotel.

Look back at Angelina Jolie's famous on-screen roles

Shooting will continue over the next five days near L'Enfant Plaza, the Navy Memorial and Pennsylvania Avenue, the paper reports.

See photos of Brad and Angelina's kids - including the twins!

As Jolie works, Pitt, 45, is also keeping busy.

See photos of Brad Pitt through the years - including his early modeling shots

He met with Energy Secretary Steven Chu on Wednesday and is set to chat later today with Speaker of the House Nancy Pelosi about reconstruction efforts in New Orleans. They will pose for photos together in the Capitol Building before their 3:30 meeting.